# A Comprehensive Review of Large Language Models for Nanophotonics: From Surrogate Modeling to Autonomous Design

arXiv: https://arxiv.org/abs/2608.18279 · HTML: https://mlsanity.com/paper/2608.18279/

## Key facts

- Cited by 1 papers in the map (data through 14 Oct 2026).
- Builds on 44 of its 201 references that are in the map.
- First posted on arXiv 18 Aug 2026.

## Builds on (most cited first, 30 of 44)

- [Attention Is All You Need](https://mlsanity.com/paper/1706.03762/) (2017)
- [An Image is Worth 16x16 Words: Transformers for Image Recognition at Scale](https://mlsanity.com/paper/2010.11929/) (2020)
- [Denoising Diffusion Probabilistic Models](https://mlsanity.com/paper/2006.11239/) (2020)
- [Swin Transformer: Hierarchical Vision Transformer using Shifted Windows](https://mlsanity.com/paper/2103.14030/) (2021)
- [Retrieval-Augmented Generation for Knowledge-Intensive NLP Tasks](https://mlsanity.com/paper/2005.11401/) (2020)
- [ReAct: Synergizing Reasoning and Acting in Language Models](https://mlsanity.com/paper/2210.03629/) (2022)
- [Evaluating Large Language Models Trained on Code](https://mlsanity.com/paper/2107.03374/) (2021)
- [Visual Instruction Tuning](https://mlsanity.com/paper/2304.08485/) (2023)
- [Scaling Laws for Neural Language Models](https://mlsanity.com/paper/2001.08361/) (2020)
- [Flamingo: a Visual Language Model for Few-Shot Learning](https://mlsanity.com/paper/2204.14198/) (2022)
- [Reflexion: Language Agents with Verbal Reinforcement Learning](https://mlsanity.com/paper/2303.11366/) (2023)
- [Toolformer: Language Models Can Teach Themselves to Use Tools](https://mlsanity.com/paper/2302.04761/) (2023)
- [On the Opportunities and Risks of Foundation Models](https://mlsanity.com/paper/2108.07258/) (2021)
- [FlashAttention: Fast and Memory-Efficient Exact Attention with IO-Awareness](https://mlsanity.com/paper/2205.14135/) (2022)
- [Self-Refine: Iterative Refinement with Self-Feedback](https://mlsanity.com/paper/2303.17651/) (2023)
- [Longformer: The Long-Document Transformer](https://mlsanity.com/paper/2004.05150/) (2020)
- [Tree of Thoughts: Deliberate Problem Solving with Large Language Models](https://mlsanity.com/paper/2305.10601/) (2023)
- [Training Compute-Optimal Large Language Models](https://mlsanity.com/paper/2203.15556/) (2022)
- [Fourier Neural Operator for Parametric Partial Differential Equations](https://mlsanity.com/paper/2010.08895/) (2020)
- [A Survey of Large Language Models](https://mlsanity.com/paper/2303.18223/) (2023)
- [Emergent Abilities of Large Language Models](https://mlsanity.com/paper/2206.07682/) (2022)
- [A Survey on Large Language Model based Autonomous Agents](https://mlsanity.com/paper/2308.11432/) (2023)
- [Retrieval-Augmented Generation for Large Language Models: A Survey](https://mlsanity.com/paper/2312.10997/) (2023)
- [AutoGen: Enabling Next-Gen LLM Applications via Multi-Agent Conversation](https://mlsanity.com/paper/2308.08155/) (2023)
- [Megatron-LM: Training Multi-Billion Parameter Language Models Using Model Parallelism](https://mlsanity.com/paper/1909.08053/) (2019)
- [Rethinking Attention with Performers](https://mlsanity.com/paper/2009.14794/) (2020)
- [GenEval: An Object-Focused Framework for Evaluating Text-to-Image Alignment](https://mlsanity.com/paper/2310.11513/) (2023)
- [A Survey on In-context Learning](https://mlsanity.com/paper/2301.00234/) (2022)
- [Parameter-Efficient Fine-Tuning for Large Models: A Comprehensive Survey](https://mlsanity.com/paper/2403.14608/) (2024)
- [Large Language Models: A Survey](https://mlsanity.com/paper/2402.06196/) (2024)

## Built on by (most cited first, 1 of 1)

- [Towards a universal meta-optics solver via large language models](https://mlsanity.com/paper/2608.26417/) (2026)

## Abstract (arXiv)

Metasurfaces have revolutionized the development of photonic devices by enabling unprecedented precision in light manipulation. However, their design processes are often constrained by computationally expensive simulations and complex high-dimensional design spaces. Although deep learning has accelerated the design process by serving as a surrogate model, it remains constrained by task-specific architectures and lacks universal reasoning capabilities. This review surveys how Large Language Models (LLMs) are adding semantic interfaces, code generation, and tool orchestration to established numerical nanophotonic workflows. We first outline the development from classical neural networks to transformer-based models and their applications in nanophotonic design. We then review the emergence of LLM-related methods in nanophotonics and organize them into two operational modes: surrogate models that treat structure-spectrum mapping as a language task, and agentic systems that have been demonstrated to generate code, orchestrate selected simulation steps, and support closed-loop optimization. Furthermore, to identify future cross-disciplinary opportunities, we briefly explore applications of LLMs in research fields such as materials science and wireless communications. This review concludes by looking ahead to the next generation of multimodal foundation models with physical perception capabilities. In this vision, artificial intelligence is evolving from passive tools into active collaborators, participating in autonomous scientific discovery.